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1 Ergebnisse
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Tuning Reactivity of Zr-Substituted Keggin Phosphotungstate..:
Nataliya V. Maksimchuk
;
Sofia M. Marikovskaya
;
Kirill P. Larionov
...
doi:10.1021/acs.inorgchem.3c02578.s001. , 1753
Link:
https://doi.org/10.1021/acs.inorgchem.3c02578.s001
RT Journal T1
Tuning Reactivity of Zr-Substituted Keggin Phosphotungstate in Alkene Epoxidation through Balancing H 2 O 2 Activation Pathways: Unusual Effect of Base
UL https://suche.suub.uni-bremen.de/peid=base-ftdeakinunifig:oai:figshare.com:article_24503927&Exemplar=1&LAN=DE A1 Nataliya V. Maksimchuk A1 Sofia M. Marikovskaya A1 Kirill P. Larionov A1 Artem A. Antonov A1 Mikhail V. Shashkov A1 Vadim V. Yanshole A1 Vasilii Yu. Evtushok A1 Oxana A. Kholdeeva YR 1753 K1 Biochemistry K1 Molecular Biology K1 Pharmacology K1 Evolutionary Biology K1 Ecology K1 Plant Biology K1 Chemical Sciences not elsewhere classified K1 sterically hindered electron K1 preferably epoxidized despite K1 including terminal ones K1 heterolytic oxidation products K1 enhancing oxygen transfer K1 also affect regioselectivity K1 n )< sub K1 active oxidizing species K1 )< K1 ooh )]< sup K1 8 –</ sup K1 4 –</ sup K1 substituted keggin phosphotungstate K1 type dimeric phosphotungstate K1 4 </ sub K1 39 </ sub K1 11 </ sub K1 31 </ sup K1 form monomeric species K1 kinetic modeling implicated K1 inert toward alkenes K1 increase substrate conversion K1 improved epoxidation selectivity K1 dimeric peroxo complexes K1 2 </ sub K1 zr }< sub K1 acid additives produce K1 oxidant utilization efficiency K1 1 </ b K1 peroxo species K1 substrate conversion K1 )}< sub K1 x </ K1 p </ K1 monosubstituted keggin K1 monomeric zr K1 2 ) K1 basic additives K1 (< b K1 various kinds K1 unusual effect K1 unproductive decomposition JF doi:10.1021/acs.inorgchem.3c02578.s001 LK http://dx.doi.org/https://doi.org/10.1021/acs.inorgchem.3c02578.s001 DO https://doi.org/10.1021/acs.inorgchem.3c02578.s001 SF ELIB - SuUB Bremen
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